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|a 9783319605319
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|a 10.1007/978-3-319-60531-9
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|a (DE-He213)978-3-319-60531-9
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|a Hepting, Matthias.
|e author.
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|4 http://id.loc.gov/vocabulary/relators/aut
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|a Ordering Phenomena in Rare-Earth Nickelate Heterostructures
|h [electronic resource] /
|c by Matthias Hepting.
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|a 1st ed. 2017.
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|a Cham :
|b Springer International Publishing :
|b Imprint: Springer,
|c 2017.
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|a XVI, 147 p. 63 illus., 56 illus. in color.
|b online resource.
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|a text
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|a Springer Theses, Recognizing Outstanding Ph.D. Research,
|x 2190-5053
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|a Springer eBook Collection
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|a Introduction: Transition Metal Oxides and their Heterostructures -- The Rare-earth Nickelates -- Experimental Techniques -- Tunable Order Parameters in Nickelate Heterostructures -- Complex Magnetic Order in Nickelate Slabs.
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|a This thesis presents an experimental study of ordering phenomena in rare-earth nickelate-based heterostructures by means of inelastic Raman light scattering and elastic resonant x-ray scattering (RXS). Further, it demonstrates that the amplitude ratio of magnetic moments at neighboring nickel sites can be accurately determined by RXS in combination with a correlated double cluster model, and controlled experimentally through structural pinning of the oxygen positions in the crystal lattice. The two key outcomes of the thesis are: (a) demonstratingfull control over the charge/bond and spin order parameters in specifically designed praseodymium nickelate heterostructures and observation of a novel spin density wave phase in absence of the charge/bond order parameter, which confirms theoretical predictions of a spin density wave phase driven by spatial confinement of the conduction electrons; and (b) assessing the thickness-induced crossover between collinear and non-collinear spin structures in neodymium nickelate slabs, which is correctly predicted by drawing on density functional theory. .
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|a Loaded electronically.
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|a Electronic access restricted to members of the Holy Cross Community.
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|a Superconductivity.
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|a Superconductors.
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|a Spectroscopy.
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|a Microscopy.
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|a Surfaces (Physics).
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|a Interfaces (Physical sciences).
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|a Thin films.
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|a Materials science.
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|a Electronic resources (E-books)
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|a Springer Theses, Recognizing Outstanding Ph.D. Research,
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